Publisher DOI: 10.1515/ijcre-2018-0166
Title: Ethylene Hydrogenation in Pellets with Different Pore Structures, Measured in a One-Sided Single-Pellet Reactor
Language: English
Authors: Argönül, Aykut 
Keil, Frerich 
Keywords: effect of pore structures on reactions;Ethylene hydrogenation;kinetic turbo reactor;one-sided single-pellet reactor;pore modelling
Issue Date: 11-Jun-2019
Source: International Journal of Chemical Reactor Engineering 6 (17): 20180166 (2019-06-11)
Journal or Series Name: International journal of chemical reactor engineering 
Abstract (english): The ethylene hydrogenation reaction was investigated in a kinetic turbo reactor and a one-sided single-pellet reactor. An empirical kinetic expression was fitted to experimental results taken from the turbo reactor, and the gas compositions at the catalyst centers were measured for three different pore structures by means of the single-pellet reactor. A bimodal pore model was developed and applied to the computation of the gas composition profiles inside the three pore structures. The calculated results were compared to the measurements. A distinct influence of the pore structures on the gas fluxes and concentration profiles inside the pores could be detected which demonstrates that the proper choice of the pellet pore structure is of importance for a high conversion.
URI: http://hdl.handle.net/11420/5537
ISSN: 2194-5748
Institute: Chemische Reaktionstechnik V-2 
Type: (wissenschaftlicher) Artikel
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