Publisher DOI: 10.1016/j.catcom.2021.106335
Title: Spatially-resolved reaction profiles in Fischer-Tropsch synthesis : influence of operating conditions and promotion for iron-based catalysts
Language: English
Authors: Wolke, Florian 
Hu, Yiwen 
Schmidt, Michael 
Korup, Oliver 
Horn, Raimund 
Reichelt, Erik 
Jahn, Matthias 
Michaelis, Alexander 
Keywords: Fischer-Tropsch synthesis;Reaction profile;Iron catalyst;In-situ analysis
Issue Date: Oct-2021
Publisher: Elsevier
Source: Catalysis Communications 158: 106335 (2021-10)
Journal: Catalysis communications 
Abstract (english): 
The complex reaction mechanism of iron-based Fischer-Tropsch synthesis comprises of manifold primary and secondary reaction pathways. Within this work, an experimental setup for spatially-resolved measurements on promoted iron-based Fischer-Tropsch catalysts is presented, allowing for a general study of the influence of operating conditions and promotion as well as of the influence of secondary reactions on product selectivity. It was found that, depending on catalyst composition, considerable hydrogenation of 1-alcohols and olefins occurs, while no influence of reinitiation of chain growth on product distribution could be found.
URI: http://hdl.handle.net/11420/9868
Institute: Chemische Reaktionstechnik V-2 
Document Type: Article
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