Publisher DOI: 10.1002/ceat.201800677
Title: Theoretical Computational Fluid Dynamics Study of the Chemical Vapor Deposition Process for the Manufacturing of a Highly Porous 3D Carbon Foam
Authors: Marx, Janik 
Berns, Jan Christoph 
Spille, Claas 
Mintken, Mona 
Adelung, Rainer 
Schlüter, Michael 
Fiedler, Bodo 
Issue Date: Jun-2019
Source: Chemical Engineering and Technology 6 (42): 1240-1246 (2019-06)
Journal or Series Name: Chemical Engineering and Technology 
Abstract (english): Aerographite is a three-dimensional carbon foam with a tetrapodal morphology. The manufacturing of aerographite is carried out in a chemical vapor deposition (CVD) process, based on a zinc oxide (ZnO) template, in which the morphology is replicated into a hollow carbon shell. During the replication process, the template is reduced by the simultaneous formation of the carbon structure. The CVD process is one of the most efficient methods for the manufacturing of various carbon nanostructures, such as graphene or carbon nanotubes (CNTs). Based on the growth mechanism of aerographite, a computational fluid dynamics model is presented for the fundamental investigations of the temperature and flow/microflow behavior during the replication process. This allows a deeper process understanding and further optimizations.
URI: http://hdl.handle.net/11420/2751
ISSN: 0930-7516
Institute: Kunststoffe und Verbundwerkstoffe M-11 
Mehrphasenströmungen V-5 
Type: (wissenschaftlicher) Artikel
Funded by: The authors gratefully acknowledge project funding by the German Research Foundation Project No. 271608950 and from the European Union's Horizon 2020 research and innovation program under grant agreement No. 78519.We would also like to thank the Federal State of Hamburg for funding this joint research project under grant No. LFF-FV 43 'New reactor technologies for chemical and biochemical synthesis processes'.
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