27 results
Now showing1 - 10 of 27
- Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: with files , Polaritonic quasi-bound states in the continuum in individual van der Waals nanoantennasThe study of strong light–matter interaction in van der Waals (vdW) materials is at the forefront of current research in physics and chemistry, and it can be enhanced dramatically by employing optical resonances. Here, we report on the first observation of quasi-bound states in the continuum (qBICs) realized via polaritonic interfering resonances in isolated WS2 nanodisks. We validate experimentally the existence of polaritonic qBICs driven by the intrinsic coupling of Mie resonances and vdW excitons. We observe exceptionally strong light–matter interaction with a measured Rabi splitting approaching 270 meV – the largest reported value among all transition metal dichalcogenide self-hybridized systems to date. The giant coupling strength stems from qBIC-induced in-plane field enhancement, which strongly interacts with in-plane excitonic dipoles while suppressing radiative losses. Polarization-controlled measurements further demonstrate selective excitation of qBIC through switching incident polarization to specific orthogonal configurations. The observed polarization-dependent coupling provides an additional degree of freedom to control the hybrid states’ spectral characteristics and spatial field distributions. Our demonstrations provide a pathway for engineering high-quality light–matter hybrid states in compact nanostructures, with potential applications in on-chip photonics, polaritonics, and quantum optics.Publicationtype: Journal Article22 4 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: with files , Integration of 2D materials in radial van der Waals heterostructure metasurfaces(American Chemical Society (ACS), 2026-05-21); ; ; ; Two-dimensional semiconductors, such as monolayer transition metal dichalcogenides (TMD), exhibit strong excitonic transitions at room temperature and offer a platform for exploring light-matter interactions in nanoscale photonic systems. In this work, we demonstrate a compact and polarization-invariant photonic metasurface, fabricated from hexagonal boron-nitride (hBN) and based on radial bound states in the continuum (BIC), which are formed by radially distributed pairs of structurally asymmetric resonators. The metasurface employs multiple symmetry-breaking perturbations to support high-quality (Q) factor resonances within a radial footprint of 4.5 μm – approximately one-sixth of the area of previous hBN BIC metasurface implementations based on large periodic arrays. Compared to these approaches, the radial geometry furthermore achieves sizable Q-factors with a reduced footprint. By integrating the hBN photonic structure with a WS2 monolayer, we observe enhanced photoluminescence when its resonance is spectrally aligned with the exciton resonance, accompanied by signatures of discrete momentum-space patterns that identify the orbital-angular-momentum-carrying ring eigenmodes. These features persist over a wide range of excitation powers and show minimal linewidth broadening, indicating robust and spatially modulated exciton-photon coupling. This work establishes a scalable approach for generating hybrid photonic-excitonic states with momentum-space structure, offering opportunities for exciton localization, valley emission, spatially programmable light-matter interaction in 2D material platforms and compact luminescent devices based on 2D material integrated metasurfaces.Publicationtype: Journal Article31 9 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Chiral nonlinear polaritonics with van der Waals metasurfaces(2026-03-27); ; ;Gryb, Dmytro ;Possmayer, ThomasChiral optical cavities are crucial for the development of nonequilibrium quantum materials by discriminating and selectively coupling to light of a specific circular polarization, but fundamentally cannot be realized with conventional mirror cavities. Here, we demonstrate this unique functionality by developing a monolithic transition metal dichalcogenide (TMDC) metasurface with broken out-of-plane symmetry, allowing for the selective formation of self-hybridized chiral exciton-polaritons. Our metasurface maintains maximal chirality for oblique incidence up to 20°, thereby outperforming all previously known designs. Moreover, we study the chiral strong-coupling regime in nonlinear experiments and reveal polaritonic signatures in chiral third-harmonic generation. Our results position maximally chiral van der Waals (vdW) metasurfaces as a versatile platform for tunable chiral polaritonics with applications in nonreciprocal photonic devices and valleytronics.Publicationtype: Journal Article21 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Spatially encoded polaritonic ultra-strong coupling in gradient metasurfaces with epsilon-near-zero modes(2025-09-12) ;Baù, Enrico ;Aigner, Andreas ;Biechteler, Jonas ;Heimig, ConnorA platform is introduced to achieve ultra-strong coupling (USC) between light and matter using widely available materials. USC is a light–matter interaction regime characterized by coupling strengths exceeding 10% of the ground state energy. It gives rise to novel physical phenomena, such as efficient single-photon coupling and quantum gates, with applications in quantum sensing, nonlinear optics, and low-threshold lasing. Although early demonstrations in plasmonic systems have been realized, achieving USC in dielectric platforms, which offer lower losses and high Q-factors, remains challenging due to typically low mode overlap between the photonic field and the material resonance. Here, dielectric dual gradient metasurfaces supporting quasi-bound-states-in-the-continuum are leveraged to spatially encode both the spectral and coupling parameter space and demonstrate USC to an epsilon-near-zero (ENZ) mode in an ultra-thin SiO₂ layer. The strong out-of-plane electric fields in tapered bar structure overlap exceptionally well with those of the ENZ mode, resulting in a normalized coupling strength of η = 0.10 and a mode splitting equivalent to 20% of the ENZ mode energy; a four-to-five-fold increase compared to previous approaches. The strong field confinement of the approach opens new possibilities for compact and scalable polaritonic devices, such as tunable frequency converters and low-energy optical modulators.Publicationtype: Journal Article23 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Ultrafast all-optical switching in nonlinear 3R-MoS₂ van der Waals metasurfaces(2025-09-02) ;Seidt, Levin; ;Seredin, Albert A. ;Possmayer, ThomasSavelev, RomanSecond-order nonlinear optical processes are fundamental to photonics, spectroscopy, and information technologies, with material platforms playing a pivotal role in advancing these applications. Here, we demonstrate the exceptional nonlinear optical properties of the van der Waals crystal 3R-MoS₂, a rhombohedral polymorph exhibiting high second-order optical susceptibility (χ⁽²⁾) and remarkable second-harmonic generation (SHG) capabilities. By designing high quality factor resonances in 3R-MoS₂ metasurfaces supporting quasi-bound states in the continuum (qBIC), we first demonstrate SHG efficiency enhancement exceeding 10². Additionally, by using degenerate pump-probe spectroscopy, we harness the C₃ᵥ system’s symmetry to realize ultrafast SHG polarization switching with near-unity modulation depth. The operation speeds are limited only by the excitation pulse duration, allowing its characterization via the nonlinear autocorrelation function. These findings establish 3R-MoS₂ as a transformative platform for nanoscale nonlinear optics, offering large conversion efficiencies and ultrafast response times for advanced pulse measurement devices, integrated photonics, and quantum technologies.Publicationtype: Journal Article15 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Optical control of resonances in temporally symmetry-broken metasurfaces(2025-08-06) ;Aigner, Andreas ;Possmayer, Thomas; ;Antonov, Alexander A.Tunability in active metasurfaces has mainly relied on shifting the resonance wavelength¹’² or increasing material losses³’⁴ to spectrally detune or quench resonant modes, respectively. However, both methods face fundamental limitations, such as a limited Q factor and near-field enhancement control and the inability to achieve resonance on–off switching by completely coupling and decoupling the mode from the far field. Here we demonstrate temporal symmetry breaking in metasurfaces through ultrafast optical pumping, providing an experimental realization of radiative-loss-driven resonance tuning, allowing resonance creation, annihilation, broadening and sharpening. To enable this temporal control, we introduce restored symmetry-protected bound states in the continuum. Even though their unit cells are geometrically asymmetric, coupling to the radiation continuum remains fully suppressed, which, in this work, is achieved by two equally strong antisymmetric dipoles. By using selective Mie-resonant pumping in parts of these unit cells, we can modify their dipole balance to create or annihilate resonances as well as tune the linewidth, amplitude and near-field enhancement, leading to potential applications in optical and quantum communications, time crystals and photonic circuits.Publicationtype: Journal Article23 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Fabrication optimization of van der Waals metasurfaces: inverse patterning boosts resonance quality factorVan der Waals (vdW) materials have garnered growing interest for use as nanophotonic building blocks that offer precise control over light-matter interaction at the nanoscale, such as optical metasurfaces hosting sharp quasi-bound states in the continuum resonances. However, traditional fabrication strategies often rely on lift-off processes, which inherently introduce imperfections in resonator shape and size distribution, ultimately limiting the resonance performance. Here, an optimized fabrication approach for vdW-metasurfaces is presented that implements inverse patterning of the etching mask, resulting in increased resonator quality solely limited by the resolution of the electron beam lithography resist and etching. Applying this inverse fabrication technique on hexagonal boron nitride (hBN), quality (Q) factors exceeding 10³ in the visible spectral range are demonstrated, significantly surpassing previous results shown by lift-off fabricated structures. Additionally, the platform's potential as a biosensor is displayed, achieving remarkable sensitivity and figure of merit of 220 in a refractive index sensing experiment. The inverse technique is applied to create chiral metasurfaces from hBN, using a two-height resonator geometry to achieve up to 50% transmittance selectivity. This inverse lithography technique paves the way toward high-performances vdW-devices with high-Q resonances, establishing hBN as a cornerstone for next-generation nanophotonic and optoelectronic devices.Publicationtype: Journal Article21 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Ultrafast tuning of radiative optical losses in quasi-bound states in the continuum(2025-06) ;Possmayer, Thomas ;Aigner, Andreas; ; Optically resonant metasurfaces provide a convenient way to enhance light-matter interactions in a confined spectral region, boosting nonlinear phenomena, sensitivity in biosensing, or spontaneous emission. Specifically, structures based on symmetry-protected quasi-bound states in the continuum (qBICs) have emerged as a popular framework to design resonant metasurfaces, as their structure does not only determine the resonance's wavelength, but also the quality-factor through the asymmetry of each unit cell [1].Publicationtype: Conference Paper15 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , Angular dispersion suppression in deeply subwavelength phonon polariton bound states in the continuum metasurfaces(Nature Publishing Group, 2025-05-16) ;Nan, Lin; ; ;Seah, Geok LengCortés, EmilianoQuasi-bound states in the continuum (qBICs) achieved through symmetry breaking in photonic metasurfaces are a powerful approach for engineering resonances with high quality factors and tunability. However, miniaturization of these devices is limited as the in-plane unit-cell size typically scales linearly with the resonant wavelength. By contrast, polariton resonators can be deeply subwavelength, offering a promising solution for achieving compact devices. Here we demonstrate that low-loss mid-infrared surface phonon polaritons enable metasurfaces supporting qBICs with unit-cell volumes up to 10⁵ times smaller than the free-space volume λ03. Using 100-nm-thick free-standing silicon carbide membranes, we achieve highly confined qBIC states with exceptional robustness against incident-angle variations, a feature unique among qBIC systems. This absence of angular dispersion enables mid-infrared vibrational sensing of thin, weakly absorbing molecular layers using a reflective objective, a method that typically degrades resonance quality in standard qBIC metasurfaces. We introduce surface-phonon-polariton-based qBICs as a platform for ultraconfined nanophotonic systems, advancing the miniaturization of mid-infrared sensors and devices for thermal radiation engineering.Publicationtype: Journal Article20 - Some of the metrics are blocked by yourconsent settings
Item type:Publication, Access status: without files , All-dielectric structural coloration empowered by bound states in the continuumThe technological requirements of low-power and high-fidelity color displays have been instrumental in driving research into advanced coloration technologies. At the forefront of these developments is the implementation of dye-free approaches, which overcome previous constraints related to color resolution and fading. Resonant dielectric nanostructures have emerged as a promising paradigm, showing great potential for high efficiency, high color saturation, wide gamut palette, and image reproduction. However, they still face limitations related to color accuracy, purity, and simultaneous brightness tunability. Here, we demonstrate an all-dielectric metasurface empowered by photonic bound states in the continuum (BICs), which supports sharp resonances throughout the visible spectral range, ideally suited for producing a wide range of structural colors. The metasurface design consists of TiO<inf>2</inf> ellipses with carefully controlled sizes and geometrical asymmetry, allowing versatile and on-demand variation of the brightness and hue of the output colors, respectively.Publicationtype: Journal Article9